गोलाकार परिरोध के तहत एक कोलाइड-बहुलक मिश्रण में प्रावस्था व्यवहार और गतिशीलता

गोलाकार परिरोध के तहत एक कोलाइड-बहुलक मिश्रण में प्रावस्था व्यवहार और गतिशीलता

Abstract:

From studies via Molecular Dynamics simulations, we report results on structure and dynamics
in mixtures of active colloids and passive polymers that are confined inside a spherical container
with a repulsive boundary. All interactions in the fully passive limit are chosen in such a way that
in equilibrium coexistence between colloid-rich and polymer-rich phases occurs. For most part of
the studies the chosen compositions give rise to Janus-like structure: nearly one side of the sphere
is occupied by the colloids and the rest by the polymers. This partially wet situation mimics
approximately a neutral wall in the fully passive scenario. Following the introduction of a velocity-
aligning activity to the colloids, the shape of the polymer-rich domain changes to that of an ellipsoid,
around the long axis of which the colloid-rich domain attains a macroscopic angular momentum.
In the steady state, the orientation of this axis evolves via diffusion, magnitude of which depends
upon the strength of activity, but only weakly.

Link: https://pubs.rsc.org/en/content/articlehtml/2023/sm/d3sm00362k