Jawaharlal Nehru Centre for Advanced Scientific Research - An Autonomous Institution

Unified phase diagram of reversible-irreversible, jamming and yielding transitions in cyclically sheared soft sphere packings

The self-organization and transitions from reversible to irreversible behavior of interacting particle assemblies—driven by externally imposed stresses or deformation—are of significant interest in understanding various phenomena in soft matter. These behaviors have been investigated across diverse systems such as colloidal suspensions, glasses, and granular materials. Depending on the density and driving regimes, such transitions are associated with yielding of amorphous solids, jamming, memory formation, and related phenomena. However, the interrelation among these behaviors has not been extensively studied.

To develop a unified view of the different regimes and transitions, we computationally investigate the response of soft-sphere assemblies to athermal cyclic-shear deformation over a broad range of densities and deformation amplitudes. Cyclic-shear deformation induces transitions from reversible to irreversible behavior in both unjammed and jammed soft-sphere packings. Well above the minimum isotropic jamming density (ϕ J), this transition corresponds to yielding.

Near the jamming point and extending up to a higher-density limit (ϕ c y c J), an unjammed phase appears between a localized absorbing phase and a diffusive, irreversible phase. This unjammed phase signals a shift of the jamming point to higher densities due to annealing and introduces a regime where shear jamming becomes feasible, even for frictionless packings.

Below ϕ J , two distinct localized states—termed point-reversible and loop-reversible—are observed. We comprehensively characterize these different regimes and the transitions between them, culminating in a unified density–shear amplitude phase diagram.

Pallabi Das, Vinutha H. A. and Srikanth Sastry, Unified phase diagram of reversible-irreversible, jamming and yielding transitions in cyclically sheared soft sphere packings. PNAS 117, 10203 (2020).